In 2018, she appeared as a contestant on the survival show Produce 48 where she represented Pledis Entertainment. She was eliminated in episode 11 after ranking 26th place. Following the conclusion of Produce 48, it was rumored that she and fellow label mate and contestant Kaeun would debut in a new girl group together.
But after Kaeun left Pledis Entertainment, plans for the group's debut fell through, and Yunjin's plans were remained to be discussed. On August 24, 2021, it was revealed that Yunjin had officially signed a contract with Source Music and would be debuting as a member of the agency's new girl group, LE SSERAFIM, in the near future. On April 9, 2022, Yunjin was introduced as the sixth and final member of LE SSERAFIM.
The group debuted on May 2, 2022 with the mini album Fearless. She debuted as a solo singer on August 9, 2022 with the digital single "Raise y_our glass". Yunjin released "I ≠ Doll" on January 9, 2023.
"Love You Twice" was released on March 14, 2023. Her fourth single, "Blessing in Disguise", was released on August 14, 2023. Yunjin was featured on GroovyRoom's "Yes or No" along with Crush.
The song was released on January 17, 2024. collaborated with Yunjin on "Stupid In Love", which was released on February 16, 2024, as part of his album Love in Stereo. On February 27, Yunjin was revealed to be featured on J-Hope's upcoming album with the collaboration single "I Don't Know".
The song and album were released on March 29. On December 29, 2024, she announced that she would be releasing the sixth digital single "Jellyfish" on December 30. However, on December 30, it was announced that the single would be postponed due to the recent crash accident.
On January 7, 2025, it was announced that the single would be released on January 10.
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